We examine the ability of a modelling system to forecast the formation and transport of ozone over Catalonia, at the NE of the Iberian Peninsula. To this end, the Community Multiscale Air Quality (CMAQ) modelling system developed by the United States Environmental Protection Agency (US EPA) and the PSU/NCAR mesoscale modelling system MM5 are coupled to a new emission model, the Numerical Emission Model for Air Quality (MNEQA). The outputs of the modelling system for the period from May to October 2008 are compared with ozone measurements at selected air-monitoring stations belonging to the Catalan Government. Results indicate a good behaviour of the model in reproducing diurnal ozone concentrations, as statistical values fall within the EPA and EU regulatory frameworks.
pp. 11-23
DOI
10.3369/tethys.2010.7.02
Entire article
- - Abdul-Wahab, S. A., Bakheit, C. S., and Al-Alawi, S. M., 2005: Principal component and multiple regression analysis in modelling of ground-level ozone and factors affecting its concentration, Environ Modell Softw, 20, 1263–1271, doi: 10.1016/j.envsoft.2004.09.001.
- - Aguirre-Basurko, E., Ibarra-Berastegui, I., and Madariaga, I., 2006: Regression and multilayer perceptron-based models to forecast hourly O3 and NO2 levels in the Bilbao area, Environ Modell Softw, 21, 430–446.
- - Appel, K. W., Gilliland, A. B., Sarwar, G., and Gilliam, R. C., 2007: Evaluation of the Community Multiscale Air Quality (CMAQ) model version 4.5: Sensitivities impacting model performance. Part I-Ozone, Atmos Environ, 41, 9603–9615.
- - Brankov, E., Henry, R. F., Civerolo, K. L., Hao, W., Rao, S. T., Misra, P. K., Bloxam, R., and Reid, N., 2003: Assessing the effects of transboundary ozone pollution between Ontario, Canada and New York, USA, Environ Pollut, 123, 403–411, doi: 10.1016/S0269-7491(03)00017-4.
- - Bravo, M., Mira, T., Soler, M. R., and Cuxart, J., 2008: Intercomparison and evaluation of MM5 and Meso-NH mesoscale models in the stable boundary layer, Bound-Layer Meteor, 128, 77–101, doi: 10.1007/s10546-008-9269-y.
- - Byung, D. W. y Ching, J. K. S., 1999: Science algorithms of the EPA Models-3 Community Multiscale Air Quality (CMAQ) Modelling System, u.S. EPA/600/R-99/030.
- - Denby, B., Larssen, S., Guerreiro, C., Douros, J., Moussiopoulos, N., Fragkou, L., Gauss, M., Olesen, H., and Miranda, A. I., 2008: Guidance on the use of models for the European air quality directive, ETC/ACC Report.
- - Dudhia, J., 1996: A multi-layer soil temperature model for MM5. Preprints, Sixth PSU/NCAR Mesoscale Model Users’ Workshop, NCAR, Boulder, CO, 49-50.
- - Dudhia, J., Gill, D., Manning, K., Wang, W., and Bruyere, C., 2004: PSU/ NCAR mesoscale modeling system tutorial class notes and user’s guide: MM5 modeling system version 3, NCAR, http://www.mmm.ucar.edu/mm5/documents/tutorial-v3-notes.html.
- - EMEP, 2007: EMEP/MMSC-W Technical Report 1/2006 ISSN 1504-6179, http://www.emep.int.
- - Gangoiti, G., Millan, M., Salvador, R., and Mantilla, E., 2001: Longrange transport and re-circulation of pollutants in the western Mediterranean during the project Regional Cycles of Air Pollution in the West-central Mediterranean Area, Atmos Environ, 35, 6267–6276.
- - Grell, G., 1993: Prognostic evaluation of assumptions used by cumulus parameterizations, Mon Weather Rev, 121, 764–787.
- - Grell, G., Dodhia, J., and Stauffer, D., 1994: A Description of the Fifth Generation Penn State/ NCAR Mesoscale Model (MM5), NCAR. Tech. Note TN-398+STR, NCAR, Boulder, CO, 117 pp.
- - Grossi, P., Thunis, P., Martilli, A., and Clappier, A., 2000: Effect of sea breeze on air pollution in the greater Athens area: Part II: Analysis of different Emissions Scenarios, J Appl Meteorol, 39, 563–575, doi: 10.1175/1520-0450(2000)039<0563:EOSBOA>2.0.CO;2.
- - Guderian, R., Tingey, D. T., and Rabe, R., 1985: Effects of photochemical oxidants on plants. Air Pollution by Photochemical Oxidants, Guderian R., Springer, Berlin, pp. 129-333.
- - Hewit, C., Lucas, P., Wellburn, A., and Fall, R., 1990: Chemistry of ozone damage to plants, Chem Ind, 15, 478–481.
- - Hogrefe, C., Rao, S. T., Kasibhatla, P., Kallos, G., Tremback, C. T., Hao,W., Sistla, G., Mathur, R., and McHenry, J., 2001: Evaluating the performance of regional-scale photochemical modelling systems: Part II- ozone predictions, Atmos Environ, 35, 4175–4188, doi: 10.1016/S1352-2310(01)00183-2.
- - Hurley, P. J., Physick, W. L., and Luhar, A. K., 2005: TAPM: a practical approach to prognostic meteorological and air pollution modelling, Environ Modell Softw, 20, 737–752, doi: 10.1016/j.envsoft.2004.04.006.
- - Jimenez, J., Baldasano, J. M., and Dabdub, D., 2003: Comparison of photochemical mechanisms for air quality modeling, Atmos Environ, 37, 4179–4194, doi: 10.1016/S1352-2310(03)00567-3.
- - Jiménez, P., Jorba, O., Parra, R., and Baldasano, J. M., 2006a: Evaluation of MM5-EMICAT2000-CMAQ performance and sensitivity in complex terrain: High-resolution application to the Northeastern Iberian Peninsula, Atmos Environ, 40, 5056–5072, doi: 10.1016/j.atmosenv.2005.12.060.
- - Jiménez, P., Lelieveld, J., and Baldasano, J. M., 2006b: Multiscale Modelling of air pollutants Dynamics in the North-Western Mediterranean Basin during a typical summertime episode, J Geophys Res, 111, D18 306.
- - Jiménez, P., Jorba, O., Baldasano, J. M., and Gassó, S., 2008: The Use of a Modelling System as a Tool for Air Quality Management: Annual High-Resolution Simulations and Evaluation, Sci Total Environ, 390, 323–340, doi: 10.1016/j.scitotenv.2007.10.025.
- - Lee, S. y Fernando, H. J. S., 2004: Evaluation of Meteorological Models MM5 and HOTMAC Using PAFEX-I Data, J Appl Meteorol, 43, 1133–1148, doi: 10.1175/1520-0450(2004)043<1133:EOMMMA>2.0.CO;2.
- - Mauzerall, D. L., Sultan, B., Kim, J., and Bradford, D., 2005: NOx emissions: variability in ozone production, resulting health damages and economic costs, Atmos Environ, 39, 2851–2866.
- - Millan, M., Mantilla, E., Salvador, R., Carratala, A., Sainz, J. M., Alonso, L., Gangoiti, G., and Navazo, M., 2000: Ozone cycles in the western Mediterranean basin: Interpretation of monitoring data in complex coastal terrain, J Appl Meteorol, 39, 487–508, doi: 10.1175/1520-0450(2000)039<0487:OCITWM>2.0.CO;2.
- - Ortega, S., Soler, M. R., Alarcón, M., and Arasa, R., 2009: MNEQA: An emissions model for photochemical simulations, Atmos Environ, 43, 3670–3681, doi: 10.1016/j.atmosenv.2009.04.046.
- - Parra, R., 2004: Desarrollo del modelo EMICAT2000 para la estimación de emisiones de contaminantes del aire en Cataluñna y su uso en modelos de dispersión fotoquímica, PhD Dissertation, Universitat Politècnica de Catalunya, Spain, phD Dissertation, http://www.tdx.cat/TDX-0803104-102139.
- - San José, R., Stohl, A., Karatzas, K., Bohler, T., James, P., and Pérez, J. L., 2005: A modelling study of an extraordinary night time ozone episode over Madrid domain, Environ Modell Softw, 20, 587–593, doi: 10.1016/j.envsoft.2004.03.009.
- - Schlink, U., Herbarth, O., Richter, M., Dorling, S., Nunnari, G., Gawley, G., and Pelikan, E., 2006: Statistical models to assess the health effects and to forecast ground level ozone, Environ Modell Softw, 21, 547–558, doi: 10.1016/j.envsoft.2004.12.002.
- - Schultz, P., 1995: An explicit cloud physics parameterization for operacional numerical weather prediction, Mon Weather Rev, 123, 3331–3343.
- - Schürmann, G. J., Algieri, A., Hedgecock, I. M., Manna, G., Pirrone, N., and Sprovieri, F., 2009: Modelling local and synoptic scale influences on ozone concentrations in a topographically complex region of Southern Italy, Atmos Environ, 43, 4424–4434, doi: 10.1016/j.atmosenv.2009.06.017.
- - Seigneur, C., Pun, B., Pai, P., Louis, J. F., Solomon, P., Emery, C., Morris, R., Zahniser, M., Worsnop, D., Koutrakis, P., White, W., and Tombach, I., 2000: Guidance for the performance evaluation of three-dimensional air quality modeling systems for particulate matter and visibility, J Air Waste Manage Assoc, 50, 588–599.
- - Serrano, E., Macias, A., and Castro, M., 1993: An improved direct method of rubber craking analysis for estimating 24-hour ozone levels, Atmos Environ, 27, 431–442.
- - Silibello, C., Calori, G., Brusasca, G., Catenacci, G., and Finzi, G., 1998: Application of a photochemical grid model to Milan metropolitan area, Atmos Environ, 32, 2025–2038, doi: 10.1016/S1352-2310(97)00208-2.
- - Sistla, G., Zhou, N., Hao, W., Ku, J. Y., and Rao, S. T., 1996: Effects of uncertainties in meteorological inputs of Urban Airshed Model predictions and ozone control strategies, Atmos Environ, 30, 2011–2025, doi: 10.1016/1352-2310(95)00268-5.
- - Sitch, S., Cox, P. M., Collins, W. J., and Huntingford, C., 2007: Indirect Radiative Forcing of Climate Change through Ozone Effects on the Land-Carbon Sink, Nature, 448, 791–794, doi: 10.1038/nature06059.
- - Sokhi, R. S., San José, R., Kitwiroon, N., Fragkou, E., Pérez, J. L., and Middleton, D. R., 2006: Prediction of ozone levels in London using the MM5-CMAQ modelling system, Environ Modell Softw, 21, 566–576, doi: 10.1016/j.envsoft.2004.07.016.
- - Soler, M. R., Hinojosa, J., Bravo, M., Pino, D., and Vilà Guerau de Arellano, J., 2004: Analyzing the basic features of different complex terrain flows by means of a Doppler Sodar and a numerical model: Some implications to air pollution problems, Meteorol Atmos Phys, 85, 141–154, doi: 10.1007/s00703-003-0041-z.
- - Troen, I. S. y Mahrt, L., 1986: A simple model of the atmospheric boundary layer; sensitivity to surface evaporation, Bound-Layer Meteor, 37, 129–148, doi: 10.1007/BF00122760 .
- - US EPA, 1991: Guideline for Regulatory Application of the Urban Airshed Model, Office of Air and Radiation, Office of Air Quality Planning and Standards, Technical Support Division, Research Triangle Park, North Carolina, US, US EPA Report No. EPA-450/4-91-013.
- - US EPA, 2005: Guidance on the use of models and other analyses in attainment demonstrations for the 8-hour ozone NAAQS, Office of Air Quality Planning and Standards, Research Triangle Park, North Carolina, US, US EPA Report No. EPA-454/R-05-002. October 2005, 128 pp.
- - US EPA, 2007: Guidance of the use of models and other analysis for demonstrating attainment of air quality goals for ozone, PM2.5 and Regional haze, US Environmental protection Agency, Research Triangle Park, North Carolina, US, EPA-454/B-07-002.
- - Vestreng, V., Rigler, E., Adams, M., Kindbom, K., Pacyna, J. M., Denier van der Gon, H., Reis, S., and Travnikov, O., 2006: Inventory review. Emission data reported to LRTAP and NEC Directive; Stage 1, 2, and 3 review; Evaluation of inventories of HMs and POPs.
- - Yarwood, G., Roa, S., Yocke, M., and Whitten, G., 2005: Updates to the carbon bond chemical mechanism: CB05, final report to the US EPA, RT-0400675, http://www.camx.com.
- - Zhang, Y., Liu, P., Pun, B., and Seigneur, C., 2006a: A Comprehensive Performance Evaluation of MM5-CMAQ for the Summer 1999 Southern Oxidants Study Episode, Part-I. Evaluation Protocols, Databases and Meteorological Predictions, Atmos Environ, 40, 4825–4838, doi: 10.1016/j.atmosenv.2005.12.043.
- - Zhang, Y., Liu, P., Queen, A., Misenis, C., Pun, B., Seigneur, C., and Wu, S. Y., 2006b: A Comprehensive Performance Evaluation of MM5-CMAQ for the Summer 1999 Southern Oxidants Study Episode, Part-II.Gas and Aerosol Predictions, Atmos Environ, 40, 4839–4855, doi: 10.1016/j.atmosenv.2005.12.048.
- - Zunckel, M., Koosailee, A., Yarwood, G., Maure, G., Venjonoka, K., van Tienhoven, A. M., and Otter, L., 2006: Modelled surface ozone over southern Africa during the Cross Border Air Pollution Impact Assessment Project, Environ Modell Softw, 21, 911–924, doi: 10.1016/j.envsoft.2005.04.004.